Innovating Silyluranium Synthetic Methods: Challenges, Advancements, And Novel Approaches

This work describes the electronic and geometric structure of molecular metal complexes involving different ligand environments. These include the Cu-redox active ligand reduction series, Tp*₂U imido and anilido transformations, Lewis base activation by Tp*₂U, silyluranium synthesis and reactivity, and electrochemistry of plutonyl.