Purdue University Graduate School
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Ye-Cheng Wang's thesis

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TOTAL SYNTHESES OF BERGAMOTANE SESQUITERPENES AND LYCOPODIUM ALKALOIDS AND COMPUTATIONAL STUDY TOWARD DIAMINATION OF ALLENES AND [2+2] SELECTIVITY

thesis
posted on 2022-10-27, 12:25 authored by Ye-Cheng Wang

Total synthesis of massarinolin A, purpurlides B, D, E, 2,3-deoxypurpurolide C, phleghenrines A and B were finished. A halogen bond promoted michael addiation was discovered during mechanism study toward diamination of allenes. Computational chemsitry study conducted toward the selectivity of 2+2 reaction supported the proposed key reaction during total synthesis of gibberellic acid 18.

Funding

NIH GM128570

NIH CA023168

NSF 2102022

NSF 1625543

History

Degree Type

  • Doctor of Philosophy

Department

  • Chemistry

Campus location

  • West Lafayette

Advisor/Supervisor/Committee Chair

Mingji Dai

Advisor/Supervisor/Committee co-chair

Christopher Uyeda

Additional Committee Member 2

Abram J. Axelrod

Additional Committee Member 3

Elizabeth I. Parkinson

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